Spin melting and refreezing driven by uniaxial compression on a dipolar hexagonal plate

We investigate freezing characteristics of a finite dipolar hexagonal plate by the Monte Carlo simulation. The hexagonal plate is cut out from a piled triangular lattice of three layers with FCC-like (ABCABC) stacking structure. In the present study an annealing simulation is performed for the dipolar plate uniaxially compressed in the direction of layer-piling. We find spin melting and refreezing driven by the uniaxial compression. Each of the melting and refreezing corresponds one-to-one with a change of the ground states induced by compression. The freezing temperatures of the ground-state orders differ significantly from each other, which gives rise to the spin melting and refreezing of the present interest. We argue that these phenomena are originated by a finite size effect combined with peculiar anisotropic nature of the dipole-dipole interaction.Comment: Proceedings of the Highly Frustrated Magnetism (HFM2006) conference. To appear in a special issue of J. Phys. Condens. Matte

Controlling orbital moment and spin orientation in CoO layers by strain

We have observed that CoO films grown on different substrates show dramatic differences in their magnetic properties. Using polarization dependent x-ray absorption spectroscopy at the Co L$_{2,3}$ edges, we revealed that the magnitude and orientation of the magnetic moments strongly depend on the strain in the films induced by the substrate. We presented a quantitative model to explain how strain together with the spin-orbit interaction determine the 3d orbital occupation, the magnetic anisotropy, as well as the spin and orbital contributions to the magnetic moments. Control over the sign and direction of the strain may therefore open new opportunities for applications in the field of exchange bias in multilayered magnetic films

Electrical Control of Dynamic Spin Splitting Induced by Exchange Interaction as Revealed by Time Resolved Kerr Rotation in a Degenerate Spin-Polarized Electron Gas

The manipulation of spin degree of freedom have been demonstrated in spin polarized electron plasma in a heterostructure by using exchange-interaction induced dynamic spin splitting rather than the Rashba and Dresselhaus types, as revealed by time resolved Kerr rotation. The measured spin splitting increases from 0.256meV to 0.559meV as the bias varies from -0.3V to -0.6V. Both the sign switch of Kerr signal and the phase reversal of Larmor precessions have been observed with biases, which all fit into the framework of exchange-interaction-induced spin splitting. The electrical control of it may provide a new effective scheme for manipulating spin-selected transport in spin FET-like devices.Comment: 8 pages, 3 figures ; added some discussion

Theory of optically forbidden d-d transitions in strongly correlated crystals

A general multiband formulation of linear and non-linear optical response functions for realistic models of correlated crystals is presented. Dipole forbidden d-d optical transitions originate from the vertex functions, which we consider assuming locality of irreducible four-leg vertex. The unified formulation for second- and third-order response functions in terms of the three-leg vertex is suitable for practical calculations in solids. We illustrate the general approach by consideration of intraatomic spin-flip contributions, with the energy of 2J, where J is a Hund exchange, in the simplest two-orbital model.Comment: 9 pages, 4 figures, to appear in J. Phys. Cond. Matte

Spin Dynamics in the Second Subband of a Quasi Two Dimensional System Studied in a Single Barrier Heterostructure by Time Resolved Kerr Rotation

By biasing a single barrier heterostructure with a 500nm-thick GaAs layer as the absorption layer, the spin dynamics for both of the first and second subband near the AlAs barrier are examined. We find that when simultaneously scanning the photon energy of both the probe and pump beams, a sign reversal of the Kerr rotation (KR) takes place as long as the probe photons break away the first subband and probe the second subband. This novel feature, while stemming from the exchange interaction, has been used to unambiguously distinguish the different spin dynamics ($T_2^{1*}$ and $T_2^{2*}$) for the first and second subbands under the different conditions by their KR signs (negative for $1^{st}$ and positive for $2^{nd}$). In the zero magnetic field, by scanning the wavelength towards the short wavelength, $T_2^{1*}$ decreases in accordance with the D'yakonov-Perel' (DP) spin decoherence mechanism. At 803nm, $T_2^{2*}$(450ps) becomes ten times longer than $T_2^{1*}$(50ps). However, the value of $T_2^{2*}$ at 803nm is roughly the same as the value of $T_2^{1*}$ at 815nm. A new feature has been disclosed at the wavelength of 811nm under the bias of -0.3V (807nm under the bias of -0.6V) that the spin coherence times ($T_2^{1*}$ and $T_2^{2*}$) and the effective $g^*$ factors ($|g^*(E1)|$ and $|g^*(E2)|$) all display a sudden change, due to the "resonant" spin exchange coupling between two spin opposite bands.Comment: 9pages, 3 figure

Spin-State Transition and Metal-Insulator Transition in La1−x_{1-x}Eux_xCoO3_3}

We present a study of the structure, the electric resistivity, the magnetic susceptibility, and the thermal expansion of La$_{1-x}$Eu$_x$CoO$_3$. LaCoO$_3$ shows a temperature-induced spin-state transition around 100 K and a metal-insulator transition around 500 K. Partial substitution of La$^{3+}$ by the smaller Eu$^{3+}$ causes chemical pressure and leads to a drastic increase of the spin gap from about 190 K in LaCoO$_3$ to about 2000 K in EuCoO$_3$, so that the spin-state transition is shifted to much higher temperatures. A combined analysis of thermal expansion and susceptibility gives evidence that the spin-state transition has to be attributed to a population of an intermediate-spin state with orbital order for $x<0.5$ and without orbital order for larger $x$. In contrast to the spin-state transition, the metal-insulator transition is shifted only moderately to higher temperatures with increasing Eu content, showing that the metal-insulator transition occurs independently from the spin-state distribution of the Co$^{3+}$ ions. Around the metal-insulator transition the magnetic susceptibility shows a similar increase for all $x$ and approaches a doping-independent value around 1000 K indicating that well above the metal-insulator transition the same spin state is approached for all $x$.Comment: 10 pages, 6 figure

Significance of myocardial tenascin-C expression in left ventricular remodelling and long-term outcome in patients with dilated cardiomyopathy

Aim Dilated cardiomyopathy (DCM) has a variety of causes, and no useful approach to predict left ventricular (LV) remodelling and long-term outcome has yet been established. Myocardial tenascin-C (TNC) is known to appear under pathological conditions, possibly to regulate cardiac remodelling. The aim of this study was to clarify the significance of myocardial TNC expression in LV remodelling and the long-term outcome in DCM. Methods and results One hundred and twenty-three consecutive DCM patients who underwent endomyocardial biopsy for initial diagnosis were studied. Expression of TNC in biopsy sections was analysed immunohistochemically to quantify the ratio of the TNC-positive area to the whole myocardial tissue area (TNC area). Clinical parameters associated with TNC area were investigated. The patients were divided into two groups based on receiver operating characteristic analysis of TNC area to predict death: high TNC group with TNC area ≥2.3% (22 patients) and low TNC group with TNC area <2.3% (101 patients). High TNC was associated with diabetes mellitus. Comparing echocardiographic findings between before and 9 months after endomyocardial biopsy, the low TNC group was associated with decreased LV end-diastolic diameter and increased LV ejection fraction, whereas the high TNC group was not. Survival analysis revealed a worse outcome in the high TNC group than in the low TNC group (P < 0.001). Multivariable Cox regression analysis revealed that TNC area was independently associated with poor outcome (HR = 1.347, P = 0.032). Conclusions Increased myocardial TNC expression was associated with worse LV remodeling and long-term outcome in DCM